Evaluation of Mechanical Properties, Corrosion Resistance, and Microstructure of an Al 1Wt%Graphene- Al2O3 Hybrid Composite Sheet Produced by Accumulative Roll Bonding

Document Type : Research Paper

Authors

Department of Materials Engineering, Shiraz Branch, Islamic Azad University, Shiraz, Iran.

10.22059/jufgnsm.2024.02.11

Abstract

In the present study, the Al/Al2O3/Graphene hybrid metal matrix composite was processed by accumulative roll bonding (ARB). A mixture of Al2O3 and Graphene (0.5 Wt% for each powder) was poured between two Al layers. The process continued up to five cycles, revealing particle-free zones and clusters in the composite's microstructure. Increasing the ARB cycles improved the distribution of reinforcing particles in the aluminum matrix. Irregular porosities appeared in the early cycles and elongated in the middle ones. SEM investigation showed that better interface bonding in the last cycles increases internal stresses, promoting aluminum matrix flow and reducing porosities, crack sizes, and debonding.
Mechanical tests such as tensile tests in RD directions, microhardness, fractography, and potentiodynamic corrosion tests in 3.5 wt-% NaCl solution have been performed to characterize the produced composites for the first time. Results showed that the tensile strength of the produced composites increases by increasing the ARB cycles and reaches the maximum value in the fifth cycle. Microhardness measurement indicated that the hardness of individual layers increases continuously by increasing the ARB cycles. The tensile fracture mode is a mixed fracture mode consisting of the cleavage and dimple rupture fracture in all cycles. The corrosion rate decreased from the first to the third ARB cycle relative to pure Aluminium alloy, arising from the presence of the inert particle and good bonding. However, it increased abruptly in the fifth cycle.

Keywords

References

  1. Tiwari JK, Mandal A, Rudra A, et al. Evaluation of mechanical and thermal properties of bilayer graphene reinforced aluminum matrix composite produced by hot accumulative roll bonding. Journal of Alloys and Compounds 2019;801:49–59.
  2. Ferreira F, Ferreira I, Camacho E, et al. Graphene oxide-reinforced aluminium-matrix nanostructured composites fabricated by accumulative roll bonding. Composites Part B: Engineering 2019;164:265–271.
  3. Volokitin A, Kuzmin S. Obtaining long products by severe plastic deformation methods: A Review. Journal of Ultrafine Grained and Nanostructured Materials 2023;56:84–98.
  4. Sarkari Khorrami M. Friction stir welding of ultrafine grained aluminum alloys: a review. Journal of Ultrafine Grained and Nanostructured Materials 2021;54:1–20.
  5. Mirzadeh H. Superplasticity of fine-grained austenitic stainless steels: A review. Journal of Ultrafine Grained and Nanostructured Materials 2023;56:27–41.
  6. Esbolat A, Panin E, Arbuz A, et al. Development of Asymmetric Rolling as a Severe Plastic Deformation Method: A Review. Journal of Ultrafine Grained and Nanostructured Materials 2022;55:97–111.
  7. Hosseini SA, Manesh HD. High-strength, high-conductivity ultra-fine grains commercial pure copper produced by ARB process. Materials and Design 2009;30:2911–2918.
  8. Ebrahimi M, Wang Q. Accumulative roll-bonding of aluminum alloys and composites: An overview of properties and performance. Journal of Materials Research and Technology 2022;19:4381–4403.
  9. Mahmoud Esmaeil Zadeh LG· RS· EJ. Microstructural Evaluation, Mechanical Properties, and Corrosion Behavior of the Al/Cu/Brass Multilayered Composite Produced by the ARB Process. Metals and Materials International 2023.
  10. Ghazanlou SI, Eghbali B, Petrov R. Microstructural evolution and strengthening mechanisms in Al7075/ graphene nano-plates/ carbon nano-tubes composite processed through accumulative roll bonding. Materials Science and Engineering: A 2021;807.
  11. Melaibari A, Fathy A, Mansouri M, et al. Experimental and numerical investigation on strengthening mechanisms of nanostructured Al-SiC composites. Journal of Alloys and Compounds 2019;774:1123–1132.
  12. Yang XY, Mei QS, Mei XM, et al. Materials Science & Engineering A Al matrix composites reinforced by high volume fraction of TiAl 3 fabricated through combined accumulative roll-bonding processes 2019;754:309–317.
  13. Omran HN, Eivani AR, Farbakhti M, et al. Tribological properties of copper-graphene (CuG) composite fabricated by accumulative roll bonding. Journal of Materials Research and Technology 2023;25:4650–4657.
  14. Ferreira FB. Microstructural and Mechanical Characterization of Graphene Oxide-Reinforced Aluminium- Matrix Nanostructured Composites fabricated by Accumulative Roll Bonding 2017.
  15. Fattahi M, Rostami M, Amirkhanlu F, et al. Fabrication of aluminum TIG welding filler rods reinforced by ZrO2/reduced graphene oxide hybrid nanoparticles via accumulative roll bonding. Diamond and Related Materials 2019;99:107518.
  16. Liu X, Wei D, Zhuang L, et al. Fabrication of high-strength graphene nanosheets/Cu composites by accumulative roll bonding. Materials Science and Engineering: A 2015;642:1–6.
  17. Ghalandari L, Tajbakhsh P. Mechanical and Corrosion Properties of Graphene Oxide-Copper Nano-composites produced by the accumulative Roll Bonding (ARB) method. Journal of New Materials 2020;11:43–60.
  18. Reihanian M, Hadadian FK, Paydar MH. Fabrication of Al–2vol% Al2O3/SiC hybrid composite via accumulative roll bonding (ARB): An investigation of the microstructure and mechanical properties. Materials Science and Engineering: A 2014;607:188–196.
  19. Toroghinejad MR, Jamaati R, Nooryan A, et al. The effect of alumina content on the mechanical properties of hybrid composites fabricated by ARB process. Ceramics International 2014;40:10489–10498.
  20. Mahdavian MM, Ghalandari L, Reihanian M. Accumulative roll bonding of multilayered Cu/Zn/Al: An evaluation of microstructure and mechanical properties. Materials Science and Engineering A 2013;579:99–107.
  21. Naseri M, Hassani A, Tajally M. An alternative method for manufacturing Al/B4C/SiC hybrid composite strips by cross accumulative roll bonding (CARB) process. Ceramics International 2015;41:13461–13469.
  22. Pirlari AJ, Emamy M, Amadeh AA, et al. Elucidating the effect of TiB 2 volume percentage on the mechanical properties and corrosion behavior of Al5083-TiB 2 composites. Journal of Materials Engineering and Performance 2019;28:6912–6920.
  23. Humphreys FJ, Matherly M. The microstructures of deformed two-phase alloys. In: Recrystallization and Related Annealing Phenomena. 2nd ed. Amsterdam: Elsevier Ltd; 2004.
  24. Reihanian M, Bagherpour E, Paydar MH. On the achievement of uniform particle distribution in metal matrix composites fabricated by accumulative roll bonding. Materials Letters 2013;91:59–62.
  25. Hosford WF. Mechanical Behavior of Materials - Second Edition. second edi. 2009.
  26. Malmir N, Alizadeh M, Pashangeh S, et al. Structural characteristics and corrosion properties of Cu/Sn–Pb composite produced by accumulative roll bonding process. Archives of Civil and Mechanical Engineering 2024;24.
  27. Mahdavian MM, Khodabandeh AR, Jafarian HR, et al. Evaluation of the macro/microstructure of Al/Cu/Sn/Ni multi-layered composite produced by accumulative-roll-bonding (ARB) and post-heat treatment. Journal of Alloys and Compounds 2022;925:166711.
  28. Azushima A, Kopp R, Korhonen A, et al. Severe plastic deformation (SPD) processes for metals. CIRP Annals - Manufacturing Technology 2008;57:716–735.
  29. Naghizadeh M, Mirzadeh H. Effects of Grain Size on Mechanical Properties and Work-Hardening Behavior of AISI 304 Austenitic Stainless Steel. Steel Research International 2019;90:1–9.
  30. Koterazawa Y. Fractography. Zairyo/Journal of the Society of Materials Science, Japan 1974;23:479–489.
  31. Liu S, Tayyebi M, Assari AH, et al. Microstructure, Texture and Tensile Properties of Nickel/Titanium Laminated Composites Produced by Cross Accumulative Roll Bonding Process. Metals and Materials International 2023;29:3630–3644.
  32. Fattah-alhosseini A, Naseri M, Alemi MHH. Corrosion behavior assessment of finely dispersed and highly uniform Al/B4C/SiC hybrid composite fabricated via accumulative roll bonding process. Journal of Manufacturing Processes 2016;22:120–126.
  33. Reihanian M, Mohammad S, Baghal L, et al. A Comparative Corrosion Study of Al/Al2O3-SiC Hybrid Composite Fabricated by Accumulative Roll Bonding ( ARB ). Journal of Ultrafine Grained and Nanostructured Materials 2016;49:29–35.
  34. Sereshki MA, Azad B, Borhani E, et al. Corrosion Behavior of Commercial Aluminum Alloy Processed by ECAP.pdf. Journal of Ultrafine Grained and Nanostructured Materials 2016;49:22–28.
  35. Zakaria HM. Microstructural and corrosion behavior of Al/SiC metal matrix composites. Ain Shams Engineering Journal 2014;5:831–838.
  36. Majidabad MA, Rezaei AR, Sabour MR, et al. Mechanical properties and pitting corrosion behavior of Al5085 alloy processed via equal channel angular pressing ( ECAP ). Journal of Ultrafine Grained and Nanostructured Materials 2023:9–14.
Journal of Ultrafine Grained and Nanostructured Materials
Volume 57, Issue 2
December 2024
Pages 222-235

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History

  • Receive Date: 20 October 2024
  • Revise Date: 12 December 2024
  • Accept Date: 15 December 2024

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